In the study, sludge from the aluminum profile factory and kaolin were used as the raw materials. Through adding ZrO2 mineralizer in different contents, Al2-xZrx+yTi1-yO5 and Al4.54Si1.46O9.73 solid solution multiphase material was prepared to effectively inhibit the decomposition of aluminum titanate solid solution and optimize high temperature property of the multiphase material. With XRD and SEM means, crystalline structure and microstructure of each sample were characterized, and properties of each sample were tested. According to experimental results, the optimal addition amount of ZrO2 mineralizer was determined to be 1.5%. Correspondingly, contents for aluminum titanate solid solution, mullite solid solution and α-Al2O3 were 70.3%, 26.8% and 2.9% respectively, bulk density was 3.20 g/cm3, degree of porosity was 5.57%, water absorption rate was 1.74%, and the once thermal shock rupture strength retention rate was 90.52%. In the study, sludge from the aluminum profile factory and kaolin were used as the raw materials. Through adding ZrO2 mineralizer in different contents, Al2-xZrx + yTi1-yO5 and Al4.54Si1.46O9.73 solid solution multiphase material was prepared effectively inhibit the decomposition of aluminum titanate solid solution and optimize high temperature property of the multiphase material. With XRD and SEM means, crystalline structure and microstructure of each sample were characterized, and properties of each sample were tested. amount of ZrO2 mineralizer was determined to be 1.5%. The bulk density was 3.20 g / cm3, degree of porosity was 70%, the content of aluminum titanate solid solution and α-Al2O3 were 70.3%, 26.8% and 2.9% respectively 5.57%, water absorption rate was 1.74%, and the once thermal shock rupture strength retention rate was 90.52%.