Ionization-induced electron injection in laser wakefield accelerators, which was recently proposed to lower the laser intensity threshold for electron trapping into the wake wave, has the drawback of generating electron beams with large and continuous energy spreads, severely limiting their future applications. Complex target designs based on separating the electron trapping and acceleration stages were proposed as the only way for getting small energy-spread electron beams. Here, based on the self-truncated ionization-injection concept which requires the use of unmatched laser–plasma parameters and by using tens of TW laser pulses focused onto a gas jet of helium mixed with low concentrations of nitrogen, we demonstrate single-stage laser wakefield acceleration of multi-hundred MeV electron bunches with energy spreads of a few percent. The experimental results are verified by PIC simulations. Ionization-induced electron injection in laser wakefield accelerators, which was recently proposed to lower the laser intensity threshold for electron trapping into the wake waves, has the drawback of generating electron beams with large and continuous energy spreads, severely limiting their future applications. Complex target designs based on separating the electron trapping and acceleration stages were proposed as the only way for getting small energy-spread electron beams. Here, based on the self-truncated ionization-injection concept which requires the use of unmatched laser-plasma parameters and by using tens of TW laser pulses focused onto a gas jet of helium mixed with low concentrations of nitrogen, we demonstrate single-stage laser wakefield acceleration of multi-hundred MeV electron bunches with energy spreads of a few percent. The experimental results are verified by PIC simulations .